Attosecond Coulomb dressing in a coherent nonlinear reflection from a metal
报告人: Hrvoje Petek (University of Pittsburgh)
报告时间: 2024年12月17日 10:00
报告地点: 物理楼W260
报告摘要:When illuminated by light, free electrons in a metal screen the applied optical field by inducing the screening charge density on the Fermi screening length scale. We consider the screening response of free electrons to an incoming optical field. They are commonly described by a theoretical cartoon but never quantitatively examined in the process of screening. We perform two photon photoemission spectroscopy as a function of the optical field strength on attosecond time scale projecting the coherently responding electrons into the photoemission continuum for electron energy, momentum, and time analysis.1 The photoemission spectra of silver in the near-UV region show a field strength-dependent transformation from Bloch bands into a delocalized electron distribution that has lost character of the single particle band structure of silver. The optical field appears to induce a phase transition from a lattice-periodic band structure to a correlated photon-electron state, Interferometric measurements show that the optical field dressed state appears and decays on sub-optical cycle, attosecond time scale. Spectroscopic evidence shows a significant role of the A2 ponderomotive/diamagnetic response of the electronic system, where A is the electromagnetic vector potential.
This is a work in progress, and your critical comments are welcome.
[1] M. Aeschlimann et al., Time-resolved photoelectron spectroscopy at surfaces, Surface Science 753,122631 (2024).10.1016/j.su
报告人简介:Prof. Hrvoje Petek obtained BS degree (1980) form MIT, and PhD degree (1985) from the University of California Berkeley both in chemistry. He worked with Keitaro Yoshihara as the National and Yamada Science Foundations postdoctoral fellow and Research Associate at the Institute of Molecular Science, Japan (1985-1992). He was a Senior Research Scientist at the Hitachi Advanced Research Laboratory (1993-2000), where he initiated research on ultrafast electron dynamics in the solid state. He is continuing this research as a Professor of Physics and RK Mellon Chair of Physics and Astronomy since 2000. Petek has been recognized with the Alexander von Humboldt Research Award (2000), Morino Award (2014), Ahmed Zewail Award in Ultrafast Science and Technology (2019), and as distinguished Scientist of the Chinese Academy of Sciences (2022). He is a Fellow of the American Physical Society, and American Academy of Arts and Sciences, the Editor-in-Chief of Progress in Surface Science, and a member of numerous advisory boards.